By P. L. Villa, S. Rapagnà (auth.), Eric G. Derouane, Jerzy Haber, Francisco Lemos, Fernando Ramôa Ribeiro, Michel Guisnet (eds.)
Light alkanes are usually immune to many different types of activation. The horizontal strategy of the current ebook covers homogeneous, heterogeneous and organic catalysis, therefore permitting readers to realize an knowledge of development and ideas in study parts diversified from their very own. The publication includes either basic chapters, giving an summary of the topic, and specialized contributions that take care of the main points and cutting-edge. a consultant record can be integrated which supplies a severe perception into present growth and discusses destiny clients and significant demanding situations.
Audience: rookies and senior researchers within the box of alkane activation. The combined theoretical and sensible procedure could be of curiosity to researchers and industrialists alike.
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Additional resources for Catalytic Activation and Functionalisation of Light Alkanes: Advances and Challenges
Reaction scheme for propane aromatization on Ga/ZSM-5 catalysts. Although the reaction sequence is frequently rationalized on the basis of a classical bifunctional mechanism, with the participation of both acidic and metallic sites, the nature and location of the metal cations and their catalytic role during propane aromatization is still being questioned [13, 14]. It is recognized that both the metallic and acidic sites need to be in close proximity for achieving high aromatization selectivity.
Leonard, J. J. A. (1987) The oxidative conversion of methane to higher hydrocarbons, Journal of Catalysis, 103, 302. 20. J and Sofranko, J. A. Si0 2, Journal of Catalysis ,103, 311-319. 21. H. ( 1991) The catalytic conversion of methane to higher hydrocarbons, Studies in Surface Science and Catalysis, 61, 3. 22. H. (1994) New Directions For the Catalytic Conversion of Methane. Final Report, November 1987-0ctober 1993. Report 94 N° GRJ94/0375; Order N° PB95-I54I83, NTIS. 23. X. and Lunsford, J.
42 Table 3. Influence of the proximity of the Ga and the acid sites for propane dehydrocyclization. MFI 29 23 20 52 8 39 I 51 15 33 1 25 3 65 7 The way of Ga incorporation (isomorphous substitution in the zeolite framework, ion exchange or wet impregnation) appears to have little effect on the final catalytic properties of Ga/H-ZSM-5 catalysts. Even similar results have been obtained when the catalyst is prepared by calcination of a physical mixture of Ga20 3 and H-ZSM-5, especially if the mixture is previously molturated [21, 22].