Download Singular and Chiral Nanoplasmonics by Svetlana Boriskina, Nikolay I. Zheludev PDF
By Svetlana Boriskina, Nikolay I. Zheludev
Plasmonics has already revolutionized molecular imaging, melanoma examine, optical communications, sensing, spectroscopy, and metamaterials improvement. This booklet is a collective attempt via numerous learn teams to push the frontiers of plasmonics learn into the rising zone of harnessing and new release of photon angular momentum on micro- and nanoscales. It deals a glimpse into the continued study efforts to increase new kinds of plasmonic vortex–pinning structures and chiral nanostructures for mild harvesting, bio(chemical) sensing, drug discovery, and nanoscale strength move.
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11) where p is a linear momentum operator, ω is a vector potential created by the dipole moment of the molecule near the MNP, p12 = 1| p |2 and finally Gω = e2 ∇ · p12 · ω02 m2 ω · p21 . 12) Each term has been well explained above. We see that this is a selfconsistent equation. 13) and QNP = Im (εm ) ω 2π ∗ dV E ωi n · E ωi n . 14) In colloidal systems, MNP-molecule complexes are floating in a solution with random orientations. 15) where the +/− signs indicate that incident beam is either LCP or RCP.
On the surface of this DNA origami object, either nine positions forming a left-handed or nine positions forming a righthanded “spiral staircase” around the cylinder were chosen. At each of these positions, the ends of the three nearest staple strands were synthesized with 15 extra bases to form a “handle” for the gold NPs. The 10 nm gold NPs in these experiments were each covered with multiple (>20) thiol-modified DNA sequences that were complementary to the handle sequence. When those particles were mixed with one of the two DNA origami cylinder versions (with left or right-handed staircase attachment positions), the handle sequences were occupied by the NPs resulting in the formation of a helix of plasmonic particles of defined chirality (Fig.
Reprinted with permission from Ref. [42]. Copyright c 2012, Rights Managed by Nature Publishing Group. a direct correspondence between the CD signal and the handedness of a helix. 1 Model: Maxwell’s Equations Incorporating a Chiral Parameter Generally speaking, the light-scattering problem of core–shell multilayer structures can be solved exactly using the Mie solution. When a chiral medium is involved, its chiral property will break September 15, 2014 12:0 PSP Book - 9in x 6in 01-Boriskina-Zheludev-c01 Electrodynamic Effects in Chiral Molecular-Plasmonic Structures the symmetry of a system and the degeneracy between RCP and LCP electromagnetic waves.