By A. D. Buckingham (auth.), S. Bratos, R. M. Pick (eds.)

This booklet has its or1g1n in a NATO summer time university geared up from June 25 to July 7 1979, in Menton, France. the aim of this faculty used to be a comparative research of some of the features of vibra­ tional spectroscopy in molecular drinks and solids. This box has been swiftly increasing within the final decade; regrettably, its improvement came about independently for drinks and for solids. In those conditions, the comparability of the fundamental suggestions and methods utilized in those branches of physics seemed as a need. The lectures given on the Menton complicated learn Institute, in addition to the enormously fruitful and full of life discussions which them proven this viewpoint. the necessity of placing jointly those lectures, within the kind of a monograph, basically seemed through the ASI and the teachers accredited to put in writing the fabric they offered on the Institute, greater because of the comments of the individuals. it's the results of this collective paintings which looks within the known Plenum Series.

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Klemperer, J. Chern. Phys. 56, 2442 (1972). R. S. Muenter, Int. Rev. Science, Phys. Chern. Series 2, Vol. D. , Butterworths, London (1975), Chap. 2. R. S. Muenter, J. Chern. Phys. 60, 2929 -(1974) . A. C. Allen, J. Chern. Phys. 51, 3286 (1969). F. Diercksen, Theor. Chern. Acta-,-21, 335 (1971). -H. Popkie, H. Kistenmacher and E. Clementi, J. Chern. Phys. 59, 1325 (1973). K. Morokuma, Acc. Chern. Res. 10,294 (1977). A. Kollman, Acc. Chern. Res. 10,365 (1977). J. A. Popl~ J. Chern. Phys. 52, 4858 (1970) i 58, 3605 (1973).

F. Diercksen, Theor. Chern. Acta-,-21, 335 (1971). -H. Popkie, H. Kistenmacher and E. Clementi, J. Chern. Phys. 59, 1325 (1973). K. Morokuma, Acc. Chern. Res. 10,294 (1977). A. Kollman, Acc. Chern. Res. 10,365 (1977). J. A. Popl~ J. Chern. Phys. 52, 4858 (1970) i 58, 3605 (1973). -D. W. H. Stillinger, J. Chern. Phys. 53, 4544 (1970). D. Buckingham-,-Trans. Faraday Soc. ~, 753 (1960). 41 INFRARED AND RAMAN STUDY OF VIBRATIONAL RELAXATION IN LIQUIDS S. Bratos Laboratoire de Physique Theorique des Liquides * Universite Pierre et Marie Curie 4, Place Jussieu, 75005 Paris (France) 1 INTRODUCTION The purpose of the present lecture course is to review infrared and spontaneous Raman studies of vibrational relaxation in liquids.

D. McLean, J. Chern. Phys. 59, 4557 (1973). J. C. A. M. Karo, J. Chern. Phys. 60, 2195 "(1974) . R. T. Pack, Atomic Data 3, 195 (1971). O. Hirschfelder, Chern. Phys. Lett. 1, 325" (1967). R. W. Bruch, InternatIonal Review of Science, Phys. Chern. Series 1, Vol. 1, Chap. 4, W. , Butterworths, London (1972). J. Gerratt, Proc. Roy. Soc. A 350, 363 (1976). A. N. Murrell, Molec. Phys. 23, 1143 (1972) . N. Murrell and G. Shaw, J. Chern. Phys. ~, 1768 (1967) . N. L. A. , Academic Press, New York (1976), Chap.

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